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Supplementary material

Input files and results for the examples described in the manual

It is explained in section 4.2 of the manual how to request a VCD and a ROA calculation for methyloxirane with DALTON and Gaussian. The input files as well as the results of the calculations can be found on this page.

DALTON

Calculations are performed at the TDHF/aug-cc-pVDZ level of theory. The wavelength of the incident light (for ROA) is 532 nm.
  • The MOLECULE input file (save)
    BASIS
    aug-cc-pVDZ
    IR/VCD or Raman/ROA for methyloxirane @ TDHF/aug-cc-pVDZ.
    
        3  0 0
            8.    1
    O001     1.5630190700    -1.4919311500    -0.4586081280
            6.    3
    C002     1.9748884300     1.1626484500    -0.1140354640
    C003    -0.2874670230    -0.0708704833     0.9244351870
    C004    -2.8563172900     0.1898548070    -0.2810475700
            1.    6
    H005     3.5434102100     1.6630858600     1.1260406200
    H006     1.8110207300     2.3089808700    -1.8197646300
    H007    -0.2942170890    -0.4821221340     2.9482978600
    H008    -2.6758333600     0.6359511330    -2.2929615100
    H009    -3.9476758400     1.6940521500     0.6363955700
    H010    -3.9274819400    -1.5742953400    -0.1052557970
    
  • The HESSIAN input file (save the compressed tarball of DALTON.HES)
  • The DALTON input file for VCD (save)
    **DALTON INPUT
    .RUN PROPERTIES
    .PRINT
       1
    **WAVE FUNCTIONS
    .HF
    *ORBITAL INPUT
    .AO DELETE
    1.0D-07
    **PROPERTIES
    .VCD
    .VIBANA
    *VIBANA
    .HESFIL
    *END OF INPUT
    
  • The DALTON input file for ROA (save)
    **DALTON INPUT
    .RUN PROPERTIES
    .WALK
    .MAX IT
        200
    .PRINT
        1
    *WALK
    .NUMERI
    .DISPLACEMENT
        0.001
    **WAVE FUNCTIONS
    .HF
    *ORBITAL INPUT
    .AO DELETE
        1.0D-07
    **START
    .VROA
    *ABALNR
    .THRESH
        1.0D-08
    .FREQUE
        1
        0.08564539532
    **EACH STEP
    .VROA
    *ABALNR
    .THRESH
        1.0D-08
    .FREQUE
        1
        0.08564539532
    **PROPERTIES
    .VROA
    .RAMAN
    .VIBANA
    *RESPON
    .THRESH
        1.0D-06
    *ABALNR
    .THRESH
        1.0D-08
    .FREQUE
        1
        0.08564539532
    *VIBANA
    .HESFIL
    **END OF DALTON INPUT
    
Save the outputs of DALTON 2.0 of the VCD and ROA calculation.

Gaussian

Calculations are performed at the B3PW91/aug-cc-pVDZ level of theory. The wavelength of the incident light (for ROA) is 532 nm.
  • The input file for VCD (save)
    %chk=meox_B3PW91_aug-cc-pVDZ_vcd.chk
    # B3PW91/aug-cc-pVDZ FREQ=VCD
    
    IR/VCD for methyloxirane @ B3PW91/aug-cc-pVDZ.
    
    0 1
    8         0.828380   -0.788115   -0.242337
    6         1.042544    0.616188   -0.058552
    6        -0.154398   -0.037430    0.484776
    6        -1.509186    0.099297   -0.148636
    1         1.873345    0.875371    0.603777
    1         0.956724    1.219018   -0.967605
    1        -0.153869   -0.258729    1.558402
    1        -1.417145    0.322465   -1.219305
    1        -2.075814    0.909146    0.333843
    1        -2.084044   -0.830679   -0.035946
    
    
  • The input file for ROA (save)
    %chk=meox_B3PW91_aug-cc-pVDZ_roa.chk
    # B3PW91/aug-cc-pVDZ FREQ=ROA CPHF=RDFREQ
    
    Raman/ROA for methyloxirane @ B3PW91/aug-cc-pVDZ.
    Wavelength of the incident light is 532 nm.
    
    0 1
    8         0.828380   -0.788115   -0.242337
    6         1.042544    0.616188   -0.058552
    6        -0.154398   -0.037430    0.484776
    6        -1.509186    0.099297   -0.148636
    1         1.873345    0.875371    0.603777
    1         0.956724    1.219018   -0.967605
    1        -0.153869   -0.258729    1.558402
    1        -1.417145    0.322465   -1.219305
    1        -2.075814    0.909146    0.333843
    1        -2.084044   -0.830679   -0.035946
    
    532nm
    
    
Save the produced formatted checkpoint files of Gaussian 03 Rev. C.01 of the VCD and ROA calculation.

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